Liquid Surface Tension Measurement by Pendant Drop Method

In the coating applications, liquid surface tension measurement is critical, which include liquid-air interfacial tension and liquid-substrate (solid) interfacial tension. Contact angle measurement is a common method for the surface tension measurement; however liquid surface tension might not be available for the measurement. Pendant drop method is a good for this purpose.

Theory

Droplet geometry; Source 1

The method is based on the calculation derived from the classic Young− Laplace equation.

Where ,

  • σ: the surface tension
  • R1 and R2: the first and second radius of curvature at point d as shown in the above figure
  • R0: the radius of curvature, apex of the drop, usually set as the origin for analysis
  • Δρ is the density difference between the liquid drop and continuous phase, e.g. air.
  • g: local gravitational acceleration
  • z: height of the point d from the horizontal axis.
source 1

where beta is form parameter, or also called Bond number (B0), which is a measure of the relative importance of gravitational forces to interfacial forces. The larger bond number, the greater gravitational contribution for the liquid droplet shape.

Measurement tool

from source 2

Testing procedure

from source 2

Take a photo of the droplet, image defination, fitting, and get the surface tension data.

Factors for accurate measurement

  • Light source must be diffused to avoid optical aberrations and spurious reflection.
  • No distortion in camera images
  • Needle must be absolutely vertical
  • No vibration
  • DROPLET size and needle diameter are very critical; try to make Worthington number, W0, close to one.

Worthington number is defined as

Source 2; note: interfacial force, surface tension (N/m)*circumference of the needle, equals to gravitational force, delta density*Volume*g

Source /Reference

  • Source 1: http://dx.doi.org/10.1016/j.jcis.2015.05.012
  • Source2: https://doi.org/10.1021/acs.jced.1c00212?rel=cite-as&ref=PDF&jav=VoR
  • kruss-scientific.com